Can you help me add songs from iTunes 11.0.1 to iPhone4S?

I have a new MacBook Air and am trying to add songs from it (iTunes 11.0.1) to iPhone4S.
However, drag & drop does nothing, which is what I had done on my PC to add songs previously. 
Note: I specifically don't want to sync my songs/libraries.  I just want to add the new stuff I uploaed to MacBook Air iTunes to my iPhone4S.
Any thoughts/help would be GREATLY appreciated.

To be fair, not the news I was hoping to hear, but I'd prefer to hear the bad news sooner rather than after expending more time and energy on a fool's errand.
I uploaded the CDs on my MacBook Air as I'm moving everything there. 
So, rather than put them on the old computer and then sync there, I'm guessing at some point I'm going to have to bite the bullet and move all my songs from PC to my Mac. 
I imagine I'll have to back up on new computer and erase in the process of putting the old songs and the new on there, getting them off my new computer.
One would hope there'd be an easier and less laborious method, especially since in my established pattern of procrastination I can see me putting this off for a while.
Anyway, thanks again for the feedback.

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