6th Gen/osx10.7/iTunes 11.0 'The ipod cannot be synced because it cannot  be found.'

Hi,
I sure do hope someone has some great ideas here - because I'm stumped.  I'm trying to sync up my husband's ipod.  Gee whiz - who knew it would be so difficult. 
Products: 
I have a 6th Gen. ipod, syncing to a Macbook Pro using OS X 10.7 on iTunes 11.0.1.  I have been successfully syncing this ipod for a few years now with no trouble - mostly music & photos.
I updated iTunes to the latest version 11.0.1 and synced the ipod.  (It should be noted that I had such a screwed up library from iTunes that I deleted the entire library and reloaded it and regenerate playlists, etc..  I was able to sync up about 1,100 songs to the ipod with no problems and only used up about 6GB of space out of a total of 16GB.)
Issue:
The trouble began when I tried to upload additional music and I received the following error... 'the ipod cannot be synced because it cannot be found'.  Which is weird since my Mac & iTunes both 'saw' the device and I was able to view uploaded content 'on this ipod' in iTunes.  It doesn't matter how much data, or what kind of data I'm trying to sync - I get the same error message.
The device reads, ''Connected - Eject before disconnecting'.  So I tried to eject the from iTunes, which shows it's disconnected there - but the icon remains on my desktop and still shows it's connected on the device.  Then I tried ejecting from my desktop - no change.  The only way to remove the device is to completely MANUALLY shut down my laptop (it hangs when I try to relaunch Finder, restart or shut down within OS). 
Troubleshooting Conducted:
I have restarted and reset the device - problem persists.  Device is fully charged.  Has the latest OS.  USB ports are operating without issue with other peripherals (external HDDs/speakers).  This does not appear to be a hardware issue (laptop and device) since both appear to be functioning properly (the device with existing content and the laptop with everything else.)
I've searched through Apple's support pages as well as community discussions and was unable to really find anything similar - please forgive me if I've overlooked something.  I'm happy to go to existing solutions.
Also of note - both my son's and my iPhones have synced with this version of iTunes remotely without any problems.
Hope I've given enough info.  I hope even more that someone may have a solution for me. 
Thank you for your time.

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