After 10.1 iTunes and 4.2 IOS on Iphone 3GS upgrade, old Outlook hang retur

After hours of fiddling at the worst possible time, I may have got some of my iphone back, but not yet all. Foolishly agreed to upgrade iTunes 10 to 10.1 on Vista 64-bit Home Premium, in order to upgrade iPhone 3GS from 4.1 to 4.2.
Firstly, iTunes wouldn't run after upgrade. Had to completely uninstall and reinstall iTunes and Apple App; Support, AND manually copy CoreVideo.dll from one folder to another.
Then the 4.2 installation failed midway and forced a complete recovery and restore.
Then (and this is the problem I now have, though worked around by temporarily disabling Contact, Cal;endar, Notes and Favourites sync - Mail already disabled) iTunes hangs Ouitlook so the post-Restore sync stalls.
As I write the sync is finally running - 4 hours of solid fiddling and googling after I started. But I will need to be able to re-sync all my Outl;ook data. I have done the Add-ins check in Outlook, so where do I go from here?

I notice that the iTunes was installed under the Program Files(x86) Folder and it runs under 32 bit mode.
It seems something wrong with the installer...

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