All of a sudden not all of my songs will sync with my iPods, why?

I to go sync both iPods today and now all of a sudden random songs will not sync with the device. They play perfectly in iTunes and this has never happened before.

When I take out the battery of the aluminum remote and then put it back the Apple TV will respond with the 3 blinking lights as if it's not paired. But after a while the Apple TV light will not blink or respond to anything from the aluminum remote. Also, the remote worked fine for over a year.
Not sure if this info suggests anything different then a faulty remote, but just wanted to check.
Thanks for your help.

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