Assigning folders and files to different physical disks OS X 10.9

My mid 2010 iMac 27 i7 quadcore, 32 GB memory has two 1 TB SSDs and several 2 to 3 TB 7200 / 5200 SATA, Firewire, LAN and USB external HDs. I would like to direct OS X 10.9 to use frequently accessed System data/images (boot, OS X, utilities and and their attendant folders and files) from SSD 1 and frequently used / accessed applications and their attendant folders and files on the second SSD 2. (I use Microsft Office Word and Excel frequently and also Windows 7 running on VMWare.) Then I would like to keep less frequently used applications and their attendant folders and files on the SATA 7200 external disk (USB 3.0 to 2.0), photos on a fourth external disk (firewire 800), music on a NAS (Raid 1, 1000Gb Ethernet), and movies on a fifth external HD (firewire 800). What I need to know is how to "assign" these various files to a physical disk. Please, I am not looking for opinions and/or guesses. I am looking for a strategy known to work and/or utilites known do set this up easily and correctly. Thanks in advance. BTW, I am a retired OS programmer and software/HW knowlegable. I have no Unix (or of course Apple OS X) programming experience, but have written and modified many other OSs. So one can be reasonably technical with me in their answers. Thanks again, Skip.

Hope this helps.
1. Empty Trash.
    http://support.apple.com/kb/PH10677
2. Start up in Safe Mode
    http://support.apple.com/kb/PH11212
3. Delete "Recovered Messages", if any.
    Hold the option key down and click "Go" menu in the Finder menu bar.
    Select "Library" from the dropdown.
    Library > Mail > V2 > Mailboxes
    Delete "Recovered Messages", if any.
    Empty Trash. Restart.
4. Repair Disk
    Steps 1 through 7
    http://support.apple.com/kb/PH5836
5. Disk space / Time Machine ?/ Local Snapshots
   http://support.apple.com/kb/ht4878
6. Re-index Macintosh HD
   System Preferences > Spotlight > Privacy
   http://support.apple.com/kb/ht2409

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