Can i keep documents on a separate hard drive than Lion OS X

I have a 2011 MBP 17". On the internal spinning disk (750GB) I was running Snow Leopard. I installed a data doubler kit from OWC, taking out the optical drive and replacing it with a 120GB SSD. I then installed Lion onto that SSD and migrated my Home folder onto that drive.
On the 750 GB drive I have a Bootcamp Partition and some documents that didn't fit on the new drive.
My questions are:
1) How do I safely remove the Snow Leopard files from the original drive?
2) Can I move all of my Documents back to the larger hard drive without causing any OS problems?
Any guidance would be appreciated.

Any place where I can get a step by step instructions on how to do this? Right now there are still active users in the Snow Leopard boot disk.
What I would like to do is create a storage folder on the HDD that is an extension of my SSD User, and copy any remaining documents from the Snow Leopard user to the SSD User's folder on the HDD. Then delete all of the users on the HDD and remove the Snow Leopard files.

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http://eshop.macsales.com/item/Seagate/ST3000DM001R/
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Can i keep documents on a separate hard drive than Lion OS X

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