Can't play songs from iTunes library on MacBook Pro

I can't play anything from my iTunes (10.0) library on my MacBook Pro. When I try to, I get message that song could not be used as original file could not be found, and offer to locate it, and I end up with an exclamation mark against that file. Any ideas how to fix this?
PS Not having any problems syncing to iPhone and playing music from there.

Iphone will sync or manually manage with one and only one computer at a time.
Syncing or manually managing to another will indeed erase the current content and replace with the content from the new computer.

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