Can't read or write from iPod when it syncs with a big library

When I try to sync with my 50Gb size library in the iTunes installed on my iBook G4 (10.4.11), it appears "can't read or write from the ipod", in the middle of the synchronization. It starts to do the job very well, but when it has done only 6 or 8 Gb, the process got slower until it appears such message. I have iTunes 7.6 and ipod firmware 1.1. I have tried on Windows and Mac plattforms, trying all the combinations (Mac and/or Win formats) and the trouble persists. The device has only two weeks of use, and it was working perfectly until now. The problem it is the same if I do it manually (no automatic sync). I am not sure if the problem is defective hardware, does anybody have any idea or have similar problem? Thanks.

Thanks a lot for your answer. The idea of an increasing autoplaylist it is pretty good. I did it, in 5 Gb steps, and in the thrid step (10 Gb done), when it only has copied almost one Gb, the error message pop up again. Before the message appears, iTunes become slower and slower copyng each song until it stops in one song, and after a while, message appears. After, the system come down, almost blocked, and it takes a long until I can mount the ipod again. Of course, ipod restarts automatically and the songs copied in the last step are not there. I was taking care in every moment of the process, avoiding to leave the system suspend alone (and also turning off all the saving energy options). I am now pretty sure that the problem is on the device. Anyway, thank you very much for your valuable ideas.

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