Can't transfer video or audio files from computer to iPhone 4S

I've been trying to transfer songs and videos that I have on my work computer to my iPhone 4S. The computer is one of my authorized computers, and the files were previously stored on a portable drive. I moved the files into iTunes and then tried to move them to the iPhone, but am blocked from doing so.  Any thoughts?

What do you mean "blocked"?
What have you tried?
What happened?
Error message?
What did it say?
Is this the computer with which you normally sync?  Iphone will sync/manage itunes content with only one computer at a time.  Syncing/managing to another will erase the current content and replace with content from the new comuter.

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