Cannot expand 2007 iMac to 4GB - freezes

Hi all.  I have a 24-inch Mid 2007 iMac model iMac7,1 with a 2.4 GHz Intel Core 2 Duo processor and 2 GB of memory.  I purchased a pair of PNY 2 GB DDR2 PC2-5300 SODIMM memory modules.  When I replace the two 1GB modules with the two 2 GB modules, the iMac will not boot at all.  But any combination of the 1 GB and 2 GB modules except the two 2s, in any order, will boot.  So I can get 1, 2, or 3 GB but no more.  Given that it will boot with either 2 GB module, it appears the modules themselves are fine.  Apple's specs say this model supports 4 GB.  Any ideas on what the problem is here or how I can fix it?

Hi Russ,
The problem is the PNY RAM, our Macs actually will take 6 GB of good RAM...
Hardware Overview:
Model Name: iMac
Model Identifier: iMac7,1
Processor Name: Intel Core 2 Duo
Processor Speed: 2.4 GHz
Number Of Processors: 1
Total Number Of Cores: 2
L2 Cache: 4 MB
Memory: 6 GB
Bus Speed: 800 MHz
Boot ROM Version: IM71.007A.B03
SMC Version (system): 1.21f4
http://eshop.macsales.com/shop/apple/memory/iMac/Intel_Core_2_Duo
PNY problems...
https://discussions.apple.com/message/19559637#19559637
https://discussions.apple.com/message/19550892#19550892
https://discussions.apple.com/message/19365678#19365678

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          76% Microsoft Outlook
          7% ARM
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      172 MB Finder
      135 MB Microsoft Outlook
      94 MB Google Chrome
      94 MB com.apple.IconServicesAgent
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    Virtual Memory Information: ?
      158 MB Free RAM
      866 MB Active RAM
      706 MB Inactive RAM
      655 MB Wired RAM
      93.45 GB Page-ins
      3.83 GB Page-outs

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