Cannot get album to transfer onto iPhone

I have automatic synching set up in  iTunes for my entire music library.
There are two new albums I have added to iTunes and I can see them sitting in my music library and I can play them through iTunes. However every time I sync my iphone and iTunes they show no sign of transferring. I have 4GB of space for them both, more than sufficient. iTunes never gives me an error message or any sign they didnt transfer. But every time I check my phone and look them up, be it under Artist or Album name, they are not there and havet transferred.
I have the latest version of iTunes and the latest iPhone software for my 4S. I'm running Windows 7.

I have also noticed that whilst in iTunes it is removing the album I tell it too to clear space for new ones- it is not removing these from my iPhone. So iTunes tells me it has 4gb of space but all the albums I removed are not removing themselves off my iPhone.

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