Cannot share documents between On-Premises and Online Users by email invitation

We have a hybrid setup, no problems with email communications between on-premises and Microsoft Online users. We have also activated online Onedrive/sharepoint to start testing. One interesting thing is that users Online can share their documents by inviting
users who are on Microsoft Online, On-premises and outside this two systems. But the problem is with the users who are on-premises cannot share their documents by email invitation with the other users who are also on-premises, they can share the documents
with the users who are online only. When they try to share documents by email invitation they get error messages it their emailboxes saying that;
A communication failure occurred during the delivery of this message. Please try resending the message later. If the problem continues, contact your helpdesk.
Generating server: SMT947322-001.YLO001.MSOPRD.MSFT.NET
#< #5.5.0 smtp;550 Denied by policy> #SMTP#
It seems some kind of relay should be granted on my CAS servers or something like that but I am not sure of what should be added. I am just stuck as to what next step and where to start looking for the problem
Exchange 2010/2013 with Microsoft Online Office 365 Hybrid

No, just wanted to share documents using the invitation by mail in sharepoint/onedrive. We can share the documents normally without the email notification. Sorry to mention that even the users who are Online cannot share documents in sharepoint/onedrive
between themselves, so not between user on-premises and online users. For example a user selects a document in the library, click share and tick on by email, just gets an error
"#< #5.5.0 smtp;550 Denied by policy> #" , No RMS enabled yet.
Hi,
Sorry for my delay.
According to your further posting, the sending Denied cause is No RMS enabled yet. If that is the case, please activate Azure Rights Management (RMS) to check whether the issue persits.
When you activate Azure Rights Management (RMS), you turn on this feature for all rights-enabled services and applications. You must activate Rights Management before you can begin to use the information rights management (IRM) features within Office, SharePoint,
and Exchange. For details about how to activate RMS, please refer to:
http://technet.microsoft.com/en-us/library/jj658941.aspx
Regards,
Winnie Liang
TechNet Community Support

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