Cannot synch iPhone with iTunes

Recently switched from an iPhone 4S to an iPhone 5S. All of my music was on the 4S, and synced with iTunes. My son then tried to set up my new 5S and the only music that transferred over was the music that I had actually purchased on iTunes. All of the music on CDs that I had copied and placed on the 4S did not transfer over to the 5S. In addition, now iTunes only list the purchased music as well. The complete music library still resides on the 4S though. However, now I can't synch either the 4S or the 5S to iTunes.

Appointments are set almost every day, so likely that some were set about same time this occured. All appointments have a reminder set so that is likely also. Not many are recurring without an end date.
One thought is that there is likely some setting that is not correct. Have searced out all settings on phone, in Outlook and iTunes that appear to be connected to synch and to calendar but could have missed something. Need to check to see if Notes and Contacts are synching also.
thanks for your responses.

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