Error (261) when trying to backup purchases

I have a new computer with SATA HD and SATA DVD burner (lightscribe) and am having a problem backing up my library.
When I insert a blank CD or DVD and select backup... backup entire library... iTunes goes off and checks the library and starts its 'burn' but then the CD ejects and a message comes up:
"The attempt to burn a disc failed. An unknown error occured (261)."
I checked that the drive is compatible (it shows under preferences/advanced/burning) as suggested by the online support docs... and the burner works with Nero & Alcohol... and I have not had problems backing up in the past. The things that have changed recently are the new CD burner (Asus lightscribe) and upgrade to version 7.3.1 iTunes.
Can I assume that I can 'manually' backup my library by just copying the library to another hard drive ? I just copy my itunes folder off to the second drive ??
Thank you all.

same problem error 261
Microsoft Windows XP Home Edition Service Pack 2 (Build 2600)
Gateway D915GAG_
iTunes 7.3.1.3
CD Driver 2.0.6.1
CD Driver DLL 2.0.6.2
LowerFilters: PxHelp20 (2.0.0.0), Pfc (2.5.0.205), AFS2K (3.1.20.0),
UpperFilters: incdrm (4.3.20.1), InCDPass (4.3.20.1), GEARAspiWDM (2.0.6.1),
Current user is an administrator.
Video Display Information:
Intel(R) 82915G Express Chipset Family
Connected Device Information:
Disk drive, WDC WD2000JD-22HBB0, Bus Type ATA, Bus Address [0,0]
Disk drive, Generic USB CF Reader USB Device, Bus Type USB
Disk drive, Generic USB MS Reader USB Device, Bus Type USB
Disk drive, Generic USB SD Reader USB Device, Bus Type USB
Disk drive, Generic USB SM Reader USB Device, Bus Type USB
Disk drive, HP USB Device, Bus Type USB
CD-ROM Drive, HL-DT-ST CD-ROM GCR-8483B, Bus Type ATA, Bus Address [1,0]
CD-ROM Drive, _NEC DVD_RW ND-2510A, Bus Type ATA, Bus Address [0,0]
If you have multiple drives on the same IDE or SCSI bus, these drives may interfere with each other.
Some computers need an update to the ATA or IDE bus driver, or Intel chipset. If iTunes has problems recognizing CDs or hanging or crashing while importing or burning CDs, check the support site for the manufacturer of your computer or motherboard.
D: _NEC DVD_RW ND-2510A, Rev 2.0T
Audio CD in drive.
Found 9 songs on CD, playing time 39:59 on Audio CD.
Track 1, start time 00:02:00
Track 2, start time 03:53:72
Track 3, start time 07:06:67
Track 4, start time 09:45:50
Track 5, start time 12:37:40
Track 6, start time 18:24:17
Track 7, start time 21:42:30
Track 8, start time 28:40:20
Track 9, start time 34:33:60
Audio CD reading succeeded.
Get drive speed succeeded.
The drive CDR speeds are: 4 8 16 20 24 32.
The drive CDRW speeds are: 4.
The drive DVDR speeds are: 4.
The drive DVDRW speeds are: 4.
E: HL-DT-ST CD-ROM GCR-8483B, Rev 1.00
Drive is empty.
The last failed data CD or DVD burn had error code 261(0x00000105). It happened on drive D: _NEC DVD_RW ND-2510A on CDR media at speed 0X.

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