How do I stop iSync from attempting to sync to a phone that no longer exists?

I recently graduated to an iPhone 4S.  I use iTunes excusively for syncing to that phone.
My previous phone was a Sony Ericsson k850 (very similar to W850) and I was able to use iSync somewhat successfully.
Now, whenever I do a sync through iTunes for the 4S, iSync starts up and says it can't locate the k850.
If I go to the option and Uncheck "Enable Syncing on this computer" under iSync/Preferences/General, iTunes get all upset that synchronization has been turned off. I do not have the option to Remove the one andonly device - that choice is grayed out.
Any help appreciated.
Thanks

I don't know if this helps much, but Address Book was basically the same application in a previous version of the Mac OS. Folks still seem to use the terms interchangably though. Similarly, Calendar used to be "iCal."
I believe syncing contacts with Google or iCloud is an either/or proposition - you can't do both. When you sync with either, a copy is saved to your Mac for faster access (like a web browser's cache). I believe there's still an option to save contacts exclusively to your Mac (HD), but I don't think it's either preferred or occurs by default if you have an account such as Gmail/google or iCloud already set up.
I've never played with preferences in Contacts (Address Book), but I do have both google and iCloud accounts associated with my Mac. Under System Preferences:Mail, Contacts & Calendars, you can specify what accounts do on your Mac. If you have multiple accounts set up, a list will appear on the left side. As you select each one, a list of check boxes appear to the right for each service you want to associate with that account. For example, I have an iCloud account for mail, calendars, contacts, and Safari (among others). I have a Gmail account for mail, although it gives me the option of using this account for calendars, etc. For Gmail, the only item I have checked is mail. It's never asked me if I wanted to sync my addresses with Google.
I hope this helps... at least a little. If nothing else, I hope I've solved the "Address Book" mystery ;-)

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