HT204053 I have one ID for my phone and different ID for my iPod

But on one of the devices I cannot make purchases it just says contact iTunes support

You can contact iTunes support via this page and ask them why you are getting the message and how to resolve it (these are user-to-user forums) : http://www.apple.com/support/itunes/contact/ - click on Contact iTunes Store Support on the right-hand side of the page

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