I can not sync the song I deleted in iOS again to my iPhone

I deleted a song from my iPhone 4, in iOS 5.0.1. When I sync this song to my iPhone 4 next time, I can NOT find it any more! I tried to sync the song individually or sync the whole album, but I still can not find the song... I just want to listen to this song agian. How can I sync this song to my iPhone again? Is this a bug for iOS?

Yes, the file extension is M4R.  Does it matter where I save these files on my Macbook?  I then opened them in Itunes and played them.  I did find the Tones folder in Itunes but the Tones or Ringtones tab does not show up when I select Iphone (within Itunes).  When I open the Tones folder in the Library, it is empty.  Thanks in advance for your help.

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