I can't eject my external hard drive

Trying to transfer files from external hard drive to macbook. Downloading photos has stopped, no photos downloaded and the window with the download message is frozen to my screen. When I try to eject the hd I get this message:The volume can’t be ejected because it’s currently in use.

Ok, the unmount button is blue but won't unmount because:
The disk “My Passport” could not be unmounted.
Make sure that all applications and files are closed on this disk.
It is stuck copying pictures folder from external hard drive to macbook even though I have clicked the stop button. This is what I need to close. thanks for link to Safe Boot and thanks for your help.  If reboot will help I will try that a bit later when I have time.

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