I can't sync my ipod to my itunes library held on my external hard drive

I'm having trouble syncing my ipod (colour 20GB) to my I-tunes library. I moved to Australia, got a new laptop and brought my I-tunes library from the UK on my external hard drive. I've installed I-tunes on my new laptop here, and linked I-tunes to the external hard drive. All of the songs appear on my I-tunes library as on my previous computer when I open I-tunes, but when I connect my I-pod it does not sync to the I-tunes library. I've updated the software on the I-pod to the latest software, and I'm running the latest I-tunes on my computer. When I right click on the Ipod icon in Itunes and hit "sync" nothing happens.
I don't understand as the songs on my external hard drive are all in Itunes format, I used it at home and it worked without any problems. Is it because my Ipod is somehow still synced to my old laptop?
I have tried copying all of the songs to my local hard drive, and manually dragging and dropping tunes from the I-tunes library to my Ipod using I-tunes but nothing works.
Incredibly frustrating as I can't add or remove any songs to/from my Ipod! Can anyone help me I'm at my wits end!
IBM T60   Windows XP  

Sync Session Failed to Start iTouch iOS5: Apple Support Communities
iphone could not be synced sync session failed to start...: Apple Support Communities
and
Can't connect to the iTunes Store

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