I copied my entire iTunes folder to my new Mac and now new playlists won't sync to my iPhone.

Hi. I recently installed a new hard drive to my Macbook Pro and as I wanted a clean start decided not to restore from Time Machine. I just copied the entire old iTunes folder into my new music library. iTunes itself functions normally but it won't sync new playlists to my iPhone 5.
I had similar problems with syncing my iPhoto library to my iPhone through iTunes but I rebuilt the iPhoto library and that seemed to fix it. Is there a way to rebuild the iTunes library? I used this document:
http://support.apple.com/kb/HT1451?viewlocale=en_US&locale=en_US
and was given error code -50 saying it was unable to import the playlists.
Any help greatly appreciated.
Max

Hi. I recently installed a new hard drive to my Macbook Pro and as I wanted a clean start decided not to restore from Time Machine. I just copied the entire old iTunes folder into my new music library. iTunes itself functions normally but it won't sync new playlists to my iPhone 5.
I had similar problems with syncing my iPhoto library to my iPhone through iTunes but I rebuilt the iPhoto library and that seemed to fix it. Is there a way to rebuild the iTunes library? I used this document:
http://support.apple.com/kb/HT1451?viewlocale=en_US&locale=en_US
and was given error code -50 saying it was unable to import the playlists.
Any help greatly appreciated.
Max

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