I got a new SSD and I cannot put anything onto my iPhone 4S through the SSD, but I can on my old HDD. How can I fix this issue?

So recently I purchased a 250g SSD for my new build, while still keeping my old 1TB HDD. Whenver I try to use iTunes (the latest), I cannot transfer ANYTHING onto my iPhone 4S. There is no "Add to" button, nor can I drag and drop. However, I can do both on my old HDD. I also own an iPad 4, which I can easily use on both drives. This is quite annoying because I have to restart my computer just to add music or videos, etc. I do not want to sync because I will lose all of my music, or whatever else it takes, and I do not want that.
So how can I enable file transferring on my new SSD?

Move the ENTIRE iTunes folder from the old computer to the new computer, or drives in this case.
iDevices are designed to only sync to one library (computer).  Attempts to sync with a new library will require removing all media from the device and replacing with media from the new library.

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