I have the 20gb iPod that I need to put music back onto with my new computer. It starts to sync then it says "ITunes could not copy the song to the iPod because the file could not be read or written. ????

I have a 20gb iPod that needs music from ITunes. On my new computer I am trying to sync but I get error message "could not copy to iPod because file could not be read or written. Attempting to copy to the disk failed. The disk could not be read from or written to." I have tried several times and have reset to factory settings.

Is the new PC running XP as well, Chalotte?
If so, I might start with the following document (your error message is a possible symptom of the issue too):
iTunes displays -50 error message when syncing iPod on Windows XP

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