I have used all the storage on my iPhone 4S...can I move all my photos to iCloud?

I have used up all my storage on my iPhone 4S, because I have a lot of photos that sync from my computer, a Mac with OSX 10.9.5.  Can I take the photos off my phone, and then stop the ones on my computer from syncing back to my phone?

Greetings LOLKimmy,
Welcome to the Apple Support Communities!
I understand that you would like to import your photos that have on your iPhone to your Mac and stop iTunes from syncing your photo albums from your Mac back to your iPhone. To accomplish this, I would first suggest importing your photos to your Mac using the instructions located in the article below.
iPhoto 9.5: Import photos or video from a digital camera
After your pictures have been imported and you would like to removed your synced photos and albums from you iPhone, please follow the instructions located in the next attached article.
Sync photos to your iPhone, iPad, and iPod touch in iTunes - Apple Support
Delete synced photos
In iTunes, locate and click on your device.
Click Photos.
Choose "Selected albums" and deselect the albums or collections you want to delete.
To delete all synced photos, deselect "Sync Photos from" and, when asked, click "Remove photos."
Click Apply.
Learn how to delete photos and video synced from iTunes when you can't access the originals.
Cheers,
Joe

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