I registered for Sync and synched my settings, but Sync won't open and I cannot get the code for the other computer.

Nevermind -- problem solved! I had to go through Tools --> Options. Didn't see that on any of the FAQs or How-Tos....
-Kerry

What do you mean by "won't pick up the songs"?
You can only sync with one iTunes library. However, you can manage mauic and videos among different computer by:
Using iPhone, iPad, or iPod with multiple computers
You can transfer iTunes purchases to a computer by:
iTunes Store: Transferring purchases from your iOS device or iPod to a computer

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