I've imported a CD to my iTunes account, but how do I get those same songs onto my iPod?

I've tried to sync my accounts, but that doesn't work. Also, I know that the songs imported correctly and play because I checked my iTunes Library to make sure they did not magically disappear. I have iTunes 11.1.1 downloaded.

Also, it might be helpful to mention that anytime I make a purchase on the iTunes Store, those do get downloaded automatically to my iPod.

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