IPod 5th gen hangs up iTunes

I have a 5th generation iPod that, when attached to my Mac G4 (OS 10.5.8) causes iTunes to hang with the spinning beach ball of doom, until forced quit. The iPod will show up on the desktop, and I can move (copy) files to and from the iPod.
I tried the troubleshooting tips as per Apples articles. Also tried putting the iPod in "disk mode" but can't get it to work. I can reset the iPod, and it works fine from the wheel.
I should also add that the problems started when I was connecting to a different computer and iTunes started to sync to my iPod, then froze. Now all of my music / media is no longer on the iPod. (It was all on iTunes so I should have no problem restoring the media, if I could get it to sync)
Thanks in advance for any assistance.

This is the procedure for Disk Mode
http://support.apple.com/kb/HT1363
However, since you say you can copy files to it from the Desktop (like it was a hard drive), I'm not sure if putting it into Disk Mode will help.
And just to confirm, this is the procedure you used to reset the iPod
http://support.apple.com/kb/HT1320
I'm thinking that the hard drive volume in the iPod became corrupted when it was connected to the other computer and "started to sync to my iPod, then froze."  It's also possible that these problems, when you connected it to the other computer and the current iTunes lockup issue, is due to a hardware problem on the iPod's hard drive.
I did the following to fix a problem with an older 4th gen iPod.  IMPORTANT NOTE:  It's possible that this will not work, if there is a hardware problem on the iPod's hard drive. 
With iTunes NOT running, connect the iPod.  Run Disk Utility.  The iPod should appear in the Disk Utility sidebar, like an external hard drive.  Select the iPod's hard drive (NOT the volume indented below it) in the sidebar.  Go to the Erase tab.  Select Mac OS Extended (Journaled) as Format.  Name it anything you want.  Then, Erase it.  Hopefully, it will complete the erase, because if it does not, there may be a hardware problem on the hard drive.  And since the iPod software was just erased, it will be non-functional if a hardware problem on the iPod's hard drive prevents it from being reformatted.
When the erase completes, quit Disk Utility and run iTunes.  iTunes should recognize the iPod without locking up.  Decline any setup windows that pop up about "syncing" (choose no/cancel).  You want to get to the main iTunes window, where you can choose the iPod in the sidebar (under DEVICES) and do a Restore.  The Restore will put the latest version of software back on the iPod.  You can proceed from there and sync your music.

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