IPod cannot be synced. The disk could not be read or written to.

I have...
G5 ipod video 30Gb formated to PC
iBook G3 600MHz
iTunes 7.1 (59)
iPhoto 4.03
I use my ipod to contain all my videos, photos and music manually and nothing stored on the iBook itself, as it only has a small hard drive. I have a large amount of photos that I have in iphoto (a total of 3254 photos and 60 folders!) which I am using whilst travelling the world. I have recently started syncing photos to the ipod as a backup, also adding a copy of full res photos. This syncs fine and I have all photos on my ipod, but when I add more photos to iphoto and then plug in the ipod it will start to sync though itunes, but then will come up with an error stating "The ipod "NAME OF IPOD" cannot be synced. The disk could not be read from or written to."
The ipod still has all the photos it originally had, but not the new ones.
I have tried deleting the file that is in the library that contains the information file, this forces the ipod to re sync and start all over again with adding the photos, which it will add the new photos, but the probelm will happen again as soon as more photos are added through iphoto!
Can anyone give any advice, I really can't format the ipod and start over agaian as I will lose all my music etc and I don't have enough room to store them elsewhere!!!
Please any help please! I really need to back these files up incase something goes wrong with the computer, then I will lose all my pictures!
Help!
Thanks
Rob

Hi Rob!
First off, it might be worth upgrading to the latest iTunes version, which is 7.1(15) (or at least I think that's what it is on a Mac... for Windows, it's 7.1.1.5).
Regardless, you can install the latest version of iTunes here:
Download iTunes - 7.1.1.5
Also, if that doesn't seem to help with anything, have you seen the suggestions in this article?:
"Disk cannot be read from or written to" when syncing iPod
-Kylene

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    I get the above mssg when I try to sync a photo folder with 5th gen ipod. the music syncs just fine and the ipod is "seen" by the computer. i have enabled the disk.
    let's start with this document:
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    given that you're getting this when you try to sync photos, perhaps start by checking on the suggestion in the "Corrupt iPod photo Cache" section of the document.

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    +The iPhone cannot be synced. The disk could not be read or written to.+
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