IPod Touch "cannot be synced. The required disc cannot be found."

Yesterday, I bought 3 CD's (yep, the physical kind) and today I ripped them into iTunes on my 24" iMac (with my usual custom settings, 256kbps, stereo, 44,100 KHz, with error correction on). I had synced my iPod Touch earlier this morning. Then I went to sync my iPod Touch (2nd gen., 32GB) to get the new albums onto it (it had about 3GB of space, so shouldn't have been a problem, I thought).
However, my iPT and/or iTunes (10.3.1) started getting flaky on me. I got most of the way through syncing, but when iTunes starts transferring my Music back onto the iPT, after several tracks had been transferred to the iPT, I get a message "The iPod "[iPod's Name Here]" cannot by synced. The required disc cannot be found. When I click on the OK, iTunes shows "Finishing Sync" and then says OK to Disconnect. (?) So I try it again (several times) - some times I notice that the iPod's screen shows "Sync in Progress" even after the error message appears and I get the OK to Disconnect message after that - ? - and another time, the iPod screen (partway through syncing the music, but after syncing the apps) just goes to the charging icon with no message about syncing. I tried restarting the iPT with the 'silver' Apple logo and all - still getting errors. After some of the problems, I disconnected the USB cable from my iMac and tried unlocking the iPT's screen with my password, and then things looked sort okay - except none of the new songs show up in the Music part of my iPT.
Thinking the iPT's timing out on me, or maybe has a bad cable, I switch to a newer cable I got, but I'm still having same kinds of problems and cannot get the new albums onto the iPT. By the way, the songs play fine within iTunes, so no indication that they are garbled or such.
It's beginning to feel like my iPod Touch and/or iTunes are ptiching a fit because I didn't buy these albums from the iTMS. Verrrrrry frustrating!
Jim R.

Are you also syncing photos? If yes, try to delete the photo cache folder, explained in this article: http://support.apple.com/kb/TS1314
If this does not help, see this article for more suggestions: "Disk cannot be read from or written to" when syncing iPod or "Firmware update failure" error when updating or restoring iPod

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