Itunes 10.6.3.25 crash during sync with ipad

After installing the latest iTunes 10.6.3.25, I can no longer fully sync my iPad 2.
- after the sync has started, I see the backup complete but some time after that i will get one of a series of errors such as cannot write file to ipad, an unknown error has occured, etc.  If I try to eject the ipad, iTunes then freezes. If I use the taskmanager to close iTunes I get either a black screen with a flashing mouse cursor (which requires a power off to solve) or occassionally I can end the iTunes program via the task manager.
Syncing works fine on my iPhone 3GS.
I have already uninstalled itunes and reinstalled it - with no change in behaviour.
After trying to sync about 20 times, I have slowly managed to get about 80% of my stuff on the ipad. 
Can anyone suggest how to relove this?
Thanks.

1. Yes, you need to buy a new OS. Mac OS X 10.6 requires a Mac with an Intel CPU and at least 1GB of RAM.
2. It won't erase your files unless a problem occurs. Back up everything anyway; this can be done with Time Machine or by creating a bootable clone, and requires an external drive.
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