ITunes hangs when I try to sync with my apple devices

Hello,
I have followed troubleshooting article iTunes: May become unresponsive when connecting iPhone, iPad, or iPod touch  but this hasn't help me fix the issue.
I am running OS/X 10.9.4 and iOS 7.1.2
When I create a new user account on my MAC  the devices connect fine.  If I create another  iTunes Library on my original user account then iTunes still hangs when I connect the devices. The article doesn't describe what to do next.  What other configuration information is there that is common across both iTunes Libraries?
Thank you,

Back up all data.
Triple-click anywhere in the line below on this page to select it:
~/Library/Application Support/SyncServices
Right-click or control-click the line and select
          Services ▹ Reveal in Finder (or just Reveal)
from the contextual menu.* A folder should open with an item selected. Quit the application if it's running. Move the selected item to the Trash. Relaunch the application and test.
*If you don't see the contextual menu item, copy the selected text to the Clipboard by pressing the key combination  command-C. In the Finder, select
          Go ▹ Go to Folder...
from the menu bar and paste into the box that opens by pressing command-V. You won't see what you pasted because a line break is included. Press return.

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