ITunes Has Stopped Working on program start

Recently, whenever I open iTunes, I'm greeted with an app crash and window prompt of "iTunes has stopped working".
Problem signature:
  Problem Event Name:    APPCRASH
  Application Name:    iTunes.exe
  Application Version:    12.1.1.4
  Application Timestamp:    54de1991
  Fault Module Name:    CoreAudioToolbox.dll
  Fault Module Version:    7.9.9.6
  Fault Module Timestamp:    54ddd41b
  Exception Code:    c000001d
  Exception Offset:    00000000001fa332
  OS Version:    6.0.6002.2.2.0.256.1
  Locale ID:    1033
  Additional Information 1:    e51c
  Additional Information 2:    c3c37ca59ab88edfd3ace298e9bd9694
  Additional Information 3:    6546
  Additional Information 4:    146b18ecb7553173253bf61665dc5916
I'm also on 64bit Windows Vista.

Greetings ChrisMB95,
Welcome to the Apple Support Communities!
I understand that iTunes on your Windows computer is having an issue launching and giving you an error. In this situation, I would recommend reading over and working through the suggested troubleshooting steps in the attached article. 
iTunes for Windows Vista, Windows 7, or Windows 8: Fix unexpected quits or launch issues - Apple Support
Cheers,
Joe

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    Application Name:          iTunes.exe
    Application Version:          10.3.1.55
    Application Timestamp:          4deec351
    Fault Module Name:          MediaToolbox.dll
    Fault Module Version:          1.0.694.7
    Fault Module Timestamp:          4ddeb575
    Exception Code:          c0000005
    Exception Offset:          00250000
    OS Version:          6.0.6002.2.2.0.768.3
    Locale ID:          1033
    Additional Information 1:          fd00
    Additional Information 2:          ea6f5fe8924aaa756324d57f87834160
    Additional Information 3:          fd00
    Additional Information 4:          ea6f5fe8924aaa756324d57f87834160
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    CD Driver 2.2.0.1
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    For general advice see Troubleshooting issues with iTunes for Windows updates.
    The steps in the second box are a guide to removing everything related to iTunes and then rebuilding it which is often a good starting point unless the symptoms indicate a more specific approach. Review the other boxes and the list of support documents further down page in case one of them applies.
    Your library should be unaffected by these steps but there is backup and recovery advice elsewhere in the user tip.
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    http://support.apple.com/kb/ts1717
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    http://support.apple.com/kb/ts1717
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