ITunes message -  the sim card inserted is not supported.

i tried to unlock my iPhone 4 from orange to giffgaff using iTunes. it failed, but left me with a message that the sim card inserted is not supported. I have replaced the orange sim back in the phone, but cannot get past the message when I reconnect to iTunes. Can anyone help?
iPhone 4 is running on IOS 7.1.2

This doesn't really have anything to do with iTunes and is probably best asked of the support teams for the cards you tried to use.  Unlocking a phone is solely the purview of the carrier to whom it is locked.

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