ITunes not syncing to iPhone 4S or iPad 2

I've noticed that the music libraries on my three devices differed significantly however I have never been able to sort out the issue. 
I have a Macbook Pro(OSX 10.8.2), iTunes 11.0, an iPad 2 (6.0.1) and an iPhone 4S (6.0.1).  Each device is signed in to the same icloud account, I've read the instructions on setting up icloud so that hopefully it syncs correctly however my music libraries are vastly different.  I have home sharing turned on, and while connected to wifi I can change the library on either of the two mobile devices under "shared" to my Library and utilize the additional tunes, however when away from wifi or my MBP is closed I can not access the music. 
My question is this- in the information I read on Apple's website discussing iTunes and iCloud, it is supposed to push all new downloads to the devices logged in that do not currently have that media.  So if I purchase a song on my iPhone 4S, theoretically it should push to my MBP and iPad 2 from the way I read it.  Or am I going to have to re-sync my iPhone and iPad everytime I add a new song or album so they all have the same music library? 
This seems very redundant and a poor use for the cloud.  If that's the case, there isn't much use for iCloud in my personal opinion.
Is anyone else having this issue?

For what it is worth, when I first turned my iCloud syncing of documents on after updating to mountain lion, I encountered the same problems as yourself. Shortly after, I noticed that when I visited iCloud.com, that the iWork feature was apparently unavailable because of ongoing works. When it became available again, everything seemed to work just fine and has done so ever since. Of note, there was no other notification of these ongoing works anywhere else other than iCloud.com.

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