ITunes not syncing with my new iPhone

My new iPhone is syncing mail and calender with Exchange. However, it will not sync with iTunes. I had one successful sync and the rest of the time is says it cannot read it due to "unknown error." Has anyone had this experience? Andy suggestions?
Also, I can't seem to figure out how to access renting videos via iTunes wirelessly on my iPhone. I cannot find the category for movies or videos on the display. Any advice?
Thanks so much.

Do a restore.
You can't do videos on the iPhone version of the store-just music.

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