ITunes Store Purchase will not copy to iPhone 4

I'm a first-time community poster, so please be gentle.
I recently purchased 2 songs from iTunes Store. I continue to receive the circle-slash icon when trying to move the songs from my Music Library or the "Purchased" file on my iTunes to my iPhone 4 Music. Thank you for your time and helpful suggestions.

I just wanted to add to this as this post comes up when desperately googling for a solution.
I had the same problem, (some apps were syncing, others weren't) and I found out it was because I had moved and reorganized my Music folder and iTunes couldn't find where the app files were.
This can be checked and fixed by going into the apps menu in iTunes and clicking each app. If there is a problem, a small grey "!" will appear to the left of the name of the app. Right click the app > Get Info > Locate and navigate to the new app folder (in iTunes Media > Mobile Applications), and everything should work fine.
Hope this also helps anyone who can't find a solution that works.

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