ITunes U and iPhone synching

I want some iTunes U programs off of my iPhone.  I deleted them from iTunes U but upon synching my iPhone overwrote iTunes and placed the programs back in iTunes U.  I deleted them again and emptied the Recycle Bin.  In iTunes I clicked off Synching Books, I deleted the iTunes U programs again and emptied the Recycle Bin.  Upon clicking off Synching Books and clicking Apply...the iPhone overwrote iTunes again and the programs are back in iTunes.
I want the programs off of my iPhone but they can't be deleted unless it's done via a synch.  When I remove them from iTunes thinking that will overwrite the iPhone...the iPhone puts them back in iTunes when synching.
Help!

I'm using a Windows 7 machine and my similar problem started when I got a new iPod and tried to synch my previous iPod's library with it. What seemed to work was I located the iTunes Library.itl file in the iTunes folder and restored it to an early point. Then it recognized my iPhone as my iPhone and I was able to back-up and synch. I'm sure I'll have issues with my iPod, though.

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