Itunes will no longer sync new music to my ipod

I've had my ipod for a year and have been able to use it fine. Now, however, the ability to sync new music to my ipod has been removed. I've recently bought a new computer and successfully transferred everything over and been able to sync my ipod with the new computer and it has been working fine. THen I decided to buy some new music from the itunes store. At first I bought a few songs and placed them in a pre-existing playlist and that worked fine. Then I decided to download the next part of an audio book I bought a while ago off audible so I could listen to the next part and while I could download it it wouldn't add to itunes the way I've done it for the last 80 or so audiobooks I've downloaded from audible (go to file, select add file to library, find file, double click and then sync)
There was no error message, just when I synced it wasn't there. So I bought an album from the itunes store. Again, something I've done before. I can buy the album, I can download it, I can even make a playlist for the album and listen to it on my computer. When I sync I get no error message but nothing I try can get that album from my computer onto my ipod.
The only way I can listen to anything new (including the stuff I have already paid for) is to do so on my computer, which I don't want to do as I can't carry my computer around public transport with me. Besides, this is why I bought an ipod!
I'm not trying to do aything new, just what I've done before.
Thank you in advance!

Hi dmbnewfie,
Thank you for using the Apple Support Community. Due to the nature of your issue or question you may find more information by using another one of Apple's support resources - https://getsupport.apple.com/GetproductgroupList.action
The link below will help you redownload purchases to your computer and iPhone.
However, you may need a technical advisor to help you if the articles below don't resolve your issue:
Downloading past purchases from the iTunes Store, App Store, and iBooks Store
http://support.apple.com/kb/HT2519
iTunes: Finding lost media and downloads
http://support.apple.com/kb/ts1408
- Judy

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