Merging and storing files and folders on external hard drive

Merging and storing files/folders  - I have a MacBookPro3,1 &  a MacBookAir1,1 both running OS10.6.8 and then files from backups and archives on a LaCie 250 and LaCie 500. I want to improve my productivity by merging all files/folder into one place.
I have a WesternDigital 1T to move files/folders to and do my duplicate deletion work.
The end result I'm seeking is to have all my files/folders stored on the LaCie 500  - with space for expanding iPhoto Library and Movies then that LaCie 500 Backed up on the 1T.   As my computers are older models the internal drives are smaller - MBA 80GB and MBP160. The Air in particular gets full up quickly and doesn't work efficiently.
What steps/software have you had experience with, and would recommend to merge all my files/folders, delete duplicates, and get it all in one place - including iTunes, iPhoto. 
What are the pros and cons of keeping & working with files/folders on an external drive rather than on the internal drive?
I'm aware of sluggishness in iPhoto if the library is too large, and looked into iPhoto Library Manager as an option for my photos.
Thanks in advance for your help with this way past due Spring cleaning activity.

Plugins have to be in specific locations for the application to load them. If you're just storing plugins you're not using you can store them anywhere.

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