Moved library to new hard drive, iPod no longer communicates

Ok, I am computer savy but know next to nothing about iTunes as I don't use it, but my wife does use it. However, my wife is not computer savy.
My wife's old hard drive started dying (on a Dell laptop), so we bought a new one and moved all her files over. However, she now has 2 problems:
(1) She cannot use any of the old music files. I read around online, and I have discovered that we need to consolidate the old files from the old HD into a flash drive using the iTunes consolidate library function. Then they can be imported to the new library on the new computer. This is doable as the old drive is not yet completely dead.
(2) However, she has since purchased/downloaded new songs out of the iTunes store onto the new HD, and thus I need to keep the new HD's library intact or we'll lose the files. *Now the big problem: her iPod will not connect to the new iTunes library.* I assume this is because iPods sync with a particular library, not a particular computer, and the library of the old computer was not properly transferred. Thus there is a new library, that contains songs we don't want to lose, but we can't connect the iPod.
Please help! How do we transfer the old "library" settings that allow the iPod to be synced without completely deleting the existing library on the new hard drive?
Thanks.
OS is Windows 7 and new HD's iTunes version is 10.0.0.68.
Message was edited by: bagman27

RS
How did you go about this move?
The correct way to do it is
1. Quit iPhoto
2. Copy the iPhoto Library as an entity from your Pictures Folder to the External Disk.
3. Hold down the option (or alt) key while launching iPhoto. From the resulting menu select 'Choose Library' and navigate to the new location. From that point on this will be the default location of your library.
4. Test the library and when you're sure all is well, trash the one on your internal HD to free up space.
If you still have the original library it might be worth trying again.
Regards
TD

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tt2

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Regards
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Moved library to new hard drive, iPod no longer communicates

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