Moved picture folders around now won't sync with iPhone

I recently moved around some pictures and now most of my pictures will not sync to my iPhone.
I have tried deleting the photo cache, moving pictures into a single folder and resetting the sync history, uninstalled iTunes, restored phone, copied all my photos to another location, and each time I get an error that that my iPhone can't be read or written to or the device times out.
The strangest thing is most of the folders or pictures it doesn't seem to like were pictures that were on the phone previously or were not touched when I moved stuff around.
I am running Vista and have even tried single folders and that works for some but most error out.
Any help would be appreciated.

Hoosierbuff wrote:
I bought a concert bootleg direct from the artist
Then it is not a bootleg!
I dowloaded the songs, and now it won't sync with my iphone.  I use icloud for my songs, and I also have imatch.  WHy can't I get these songs on there?
It is possibly an incompatibility with audio format or sample rate. 
First, make sure that the songs play in iTunes on your computer.  If so, right-click and choose "create AAC version."  Use the new AAC version with your iPhone.

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