New iMac won't play many of my purchased iTunes songs

I have 2 of my 5 computers authorized for iTunes. My new iMac won't let me play many of songs, and I get a message that my iMac is not authorized to play the song I paid for on my other computer. I repeatedly go through the process of telling it my iMac is authorized...it agrees, then returns to tell me it cannot play my songs because my iMac is not authorized. What step am I missing?

Here is what customer service is now telling me to do:
I'm sorry to hear that you have been experiencing difficulties with the iTunes application. To resolve this, I recommend uninstalling and reinstalling iTunes. Before beginning, please back up your iTunes library as explained here:
How to back up your media in iTunes
http://support.apple.com/kb/HT1382
To uninstall iTunes, please follow the steps in this article:
Removing iTunes for Mac OS X
http://support.apple.com/kb/HT1224
After you've uninstalled iTunes and removed the related files, you will need to reinstall it. You can download the latest version free of charge from the iTunes website:
http://www.itunes.com/download
After you've reinstalled iTunes, please ensure you have the latest version of QuickTime installed. You can find the latest version here:
http://www.apple.com/quicktime/download
If you continue to experience difficulties with iTunes after uninstalling and reinstalling it, you may wish to call our AppleCare technical support team. A representative will be able to tell you about Apple's complimentary and fee-based support options and can help you determine which option might be most helpful in this case. To find the appropriate phone number, please visit:
http://www.apple.com/support/contact/phone_contacts.html
I hope this information has been helpful.
I havent gone through this whole process yet, has anyone else tried this yet?

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