New iPhone 4 keeps crashing my iTunes- any suggestions as to why?

I've registered my new iphone 4 with iTunes on my Mac- all fine, Apps, Contacts, iCal and so on. The music library is too large to fit so I've hit 'Automatically fill free space with songs".
Now every time I plug in it Syncs but whenever I try to do something manual in the iPhone through iTunes, it pretty much crashes it.
Any suggestions what is causing this and how I might fix it?

302jennbm wrote:
.. it says purchase can not be completed contact support iTunes. ..
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