Old Apple TVs and new Macbook

I have 3 gen 1 apple TVs and a new MacAir.  It works fine for sharing movies, but I can no longer access the disk space on my apple TVs to erase movies or add movies.  I take my laptop to work everyday, so my kids cannot watch new content when I am gone.  How do I regain access to the hard disk space on these apple tv models and erase old movies and put the new ones on so they can be watched when my computer is at work.

Welcome to the Apple Community.
Your library may have been changed from a (primary) custom syncing library to an automatic syncing library or to a (secondary) streaming library. See this.
To revert to a custom syncing library from an automatic syncing library, simply check the 'Custom Sync' radio button under the summary tab in iTunes.
To revert to a primary library from a secondary library, disconnect from the Apple TV (Settings/Computers/Your_Library) and reconnect again (Settings/Computers/Connect_to_iTunes) - You will need to re-sync previously synced content.

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