Outlook on pc. Why can't I send a new email or reply to an existing one?

I have outlook already on one pc working fine via icloud.  Also working on 2 iphones and an ipad.  What could I have done wrong when setting up the next pc which won't let me send emails or reply to them?  I have the icloud control panel and outlook 2007/windows7.  Emails from both email accounts have downloaded and continue to do so.

Nate0421, Let's make sure we get your picture messages working! What happens when you try to send a picture message from your phone to your computer? Do you receive any error messages? Are you trying to send the messages using the messaging application or via email? Please share details so we can help.
TanishaS_VZW
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