Please help Apps don't work anymore

I had set up my iphone and purchased apps on a Windows PC. All worked as it should. Changed jobs and hooked up iphone to a MAC G5. I was able to click on the iPhone icon in iTunes and do what appeared to be a copy of my apps from the iPhone to itunes using the Options key*. The icons still show up on my phone but don't work. What happens is they start to boot up and then the screen goes back to the home page. This is only an issue with downloaded apps (both free and purchased) not with the orginal apps that came on the iphone.
Please let me know if you thoughts on how to correct. Thank you,
* I think this is the key I used. I could be wrong as I am not at the Mac right now.

Since this is a new computer it may not be authorized for your account
Authorize your computer then sync to the iPhone.
This article shows you how:
http://support.apple.com/kb/HT1420

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