Problem copying files between two external drives...

Hello, and thanks for any ideas on this one.
I have a punch of .m4v video files on a 1TB Lacie external drive, but re cently bought two 3TB Seagate drives and wanted to move all these media files over to one of the new drives.  Most of the .m4v files moved just fine, but I encountered two different issues in the process that I can't resolve.
I'm on an Intel-based iMac (Core 2 Duo), running OSX 10.5.8.
1. Most pressing problem:
One of the video files, when I try to copy, causes the finder windows to completely freeze requiring a hard reboot of the machine to fix.  I can get infomation on the file OK, and can play it off the original drive just fine, but try and copy it and all manners of computer death take place.  There does not seem to be a permissions issue, and the file isn't flagged as locked.
This command produces no fruit either: $ lsof | grep videofile.m4v
2. Second issue:
This one affects two other files.  When trying to move them over, they get approx half way there and then I get a notice that the operation cannot be completed because the files are supposedly in use.
All the googling I can do on that error seems to bring up cases where files can't even start to be moved... but in these two files, they get half there.  Or maybe they're read OK but then can't write?  Either way the status bars show about 1 GIG or 1.7 copied.  I don't know.
I also checked the permissions, the locked setting, used the lsof command, etc... no luck.
About 100 other videos copied over just fine.
Any ideas are greatly appreciated.

Thanks for the response... I tried just now, no luck.
I did at least get an error this time for problem one above before the lock up... lol... error code 36.  So far searching for that isn't coming up with any solutions either. 

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