Restoration Interrupted by "Unmounted" Message

I've been having major troubles with my iPod 5th gen.
When I moved my library from my PC to my Macbook, I restored my iPod, so there is nothing on it now.
First, as I tried to sync it on my Macbook, the message "this iPod could not be synced because the disk cannot be read from or written to" came up. Then I tried to restore it, but I keep getting a message that says "this iPod could not be restored because it could not be unmounted".
I keep going through this process over and over, and nothing seems to work.
HELP!

I have little over 2500 pictures on the iPad.
I tried without a dock, used another USB-cable, even tried it without a power cable. So it shouldn't be power related.
Before I get to see the "finished loading" status, the screen goes blank and shortly the apple logo is shown.
I tried it with a single album and had no problems. I guess one "faulty" picture causes the app to crash.
I will try trough all my albums and narrow it down. Unfortunately I have quite some albums...

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