Since the latestest iTunes Update, can't sync new music

Maybe I'm doing something wrong, but as long as I purchase something from the iTunes store, it "syncs" it over the Cloud and it shows up on my iPhone 4s.  But if I move an mp3 or 4 into my iTunes, it shows up in iTunes, but not n my phone.  So, I plugged in my phone, opened iTunes, went to music, chose sync all music and pressed the sync button.  It starts to sync, I see the song I'm trying to get on my phone, but then it gets to step 5 and "hangs up" on that step forever.  I cancel the sync, but it doesn't complete the cancel.  So I quit iTunes and look at my phone, and it still has the sync circle going on it.  It won't stop, so I have to shut off my phone and restart it to get the sync symbol to stop.  The music nevers get to me phone.  Thoughts???

Thanks but I've already done that to. It has authorised the computer and tells me there are two devices authorised to use this account.  This will be because the computer was send away for a repair and came back with a new hard drive. Once I've bought the music do I have to do something with it before it will sync to phone ?
The new music seems to be in the right place and boxes are ticked but the new music won't transfer , everything else seems to be in order

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