Vista x64 and iPod Syncing Error (Error -81)

I have Vista x54 and the latest iTunes (7.1.1.5) and just got a brand-new 30GB Video 5.5 a few days ago. I started my sync on my library, but right in the middle I get this error - "Cannot Copy To Disk "IPOD" (-81)" I already restored my iPod several times and even completely removed all traces of iTunes, QT, etc and reinstalled, but to no avail... I've been using iTunes other functionalities for some time now on my Vista x64 just fine... What should I do? Is this a hardware problem - cause this iPod is spankin' new!!

Hmmm. You aren't getting the classic symptoms of the issue, but it might be worth checking for a Windows drive letter confusion on the PC, as per the following document:
Windows confuses iPod with network drive or hard drive and may keep iPod from mounting or songs may seem to disappear

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