When trying to remove a partition on my hard drive I couldn't

when trying to remove a partition on my hard drive I got an error and the option was grayed out in boot camp assistant. error message:  "The startup disk cannot be partitioned or restored to a single partition.  startup disk must be formatted as a single Mac OS Extended (Journaled) volume or already partitioned by Boot Camp Assistant for installing Window".

I am going to revise my question to this.  If I compress my itunes folder which would save me a considerable amount of space will this make the music and apps information stored in there unsyncable? 

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    B Basic information which you need to know
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